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Size-Resolved Respiratory Tract Deposition of Sub-Micrometer Aerosol Particles in a Residential Area with Wintertime Wood Combustion

机译:冬季木材燃烧小区亚微米气溶胶粒子的尺寸分辨呼吸道沉积

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摘要

Particle size distributions and hygroscopic growth were studied in a town in Sweden with extensive emissions from wood combustion. The average deposited fraction of particle number, surface area and volume dose in the human respiratory tract was estimated using the data set, as well as the typical deposition pattern of the two dominant particle source types: wood combustion and traffic exhaust. As far as we know, this is the first report on the deposited fraction and hygroscopicity of ambient particles from domestic wood combustion in the literature. The use of PM2.5 as a substitute for the deposited dose was also tested. Source/receptor modeling and the hygroscopicity measurements showed that wood combustion and traffic exhaust are dominant sources, and that these particles have a low water uptake. Number fractions of 38 and 69% of the wood combustion and traffic particles, respectively, were deposited in the respiratory tract, and 53% of the particles were deposited as an average for the whole period. The deposited fraction of the surface area and volume dose was also calculated for wood combustion particles, with the result being 22% for both parameters. The results also revealed that the PM2.5 average over more than 10 hours correlated well (r(2) > 0.80) with the deposited surface area and volume dose. This means that PM2.5 can be used as proxy for the deposited dose when examining health effect relationships during short-term exposure studies if the averaging time is sufficient, while a PM2.5 proxy is not recommended for shorter averaging times.
机译:在瑞典的一个城镇,研究了木材燃烧产生的大量排放物,研究了粒径分布和吸湿性增长。使用数据集以及两种主要颗粒源类型(木材燃烧和交通尾气)的典型沉积模式,估算了人类呼吸道中颗粒数,表面积和体积剂量的平均沉积分数。据我们所知,这是文献中有关家用木材燃烧产生的环境颗粒的沉积分数和吸湿性的第一份报告。还测试了使用PM2.5替代沉积剂量。源/受体模型和吸湿性测量表明,木材燃烧和交通尾气是主要来源,并且这些颗粒的吸水率低。在整个呼吸道中,分别有38%和69%的木材燃烧颗粒和交通颗粒沉积在呼吸道中,而53%的颗粒平均沉积在呼吸道中。还计算了木材燃烧颗粒的表面积和体积剂量的沉积分数,两个参数的结果均为22%。结果还显示,超过10小时的PM2.5平均值与沉积的表面积和体积剂量具有良好的相关性(r(2)> 0.80)。这意味着,如果平均时间足够长,则在检查短期暴露研究期间的健康影响关系时,可以将PM2.5用作沉积剂量的替代物,而对于较短的平均时间,不建议使用PM2.5替代物。

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